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    "documentation": "https://doi.org/10.5281/zenodo.14918287",
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    "funder": "https://doi.org/10.13039/501100003246",
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    {
      "project_id": "700.59.425",
      "title": "Exploiting quantum interference effects in molecular scale electronics",
      "funding_scheme_id": 798,
      "funding_scheme": "NWO-Talentprogramma Vidi 2009 CW",
      "department": "Exacte en Natuurwetenschappen",
      "sub_department": "Chemische Wetenschappen",
      "start_date": "2010-03-01T00:00:00",
      "end_date": "2015-12-31T00:00:00",
      "reporting_year": 2009,
      "summary_nl": "This project aims at the exploitation of quantum interference effects that occur on a molecular scale to obtain molecular electronic devices with improved characteristics. There is a widespread interest in the study of molecular electronics at present since the dimensions of the active element in integrated circuits are rapidly approaching those of single molecules. Although considerable progress has been made in this field, the design of molecular devices often disregards quantum interference effects that are operative on the scale of singe molecules. In this project these interference effects will be explicitly considered with the aim to use them in a functional way. In this way it will be possible to make molecular transistors with very high on/off ratios and fast switching speeds.\n\nThe interference effects will be studied by considering charge transfer in donor-bridge-acceptor systems where charge transfer occurs upon excitation with a short laser pulse. The molecular bridge will explicitly be chosen to exhibit interference effects on charge transfer. Examples of such bridges are molecules containing two separate pathways for charge transfer (a molecular Mach-Zehnder interferometer) or systems with a dangling reflecting ?stub? (molecular quantum interference transistor). Charge transfer in such systems will be studied experimentally using time-resolved spectroscopic techniques, and theoretically using quantum chemical simulations. The research proposed here will lead to a profound fundamental understanding of quantum interference effects in molecular electronics and quantitative knowledge on the effects of dephasing.\n\nThe approach of studying molecular electronic components through spectroscopic characterization of charge transfer in donor-bridge-acceptor systems represents a strong and unique addition to the considerable effort on molecular scale electronics in the Netherlands. The applicant is excellently positioned to pursue such a program given his proven track record in combining spectroscopic experimental work with computational chemistry to study charge and excited state dynamics.\n\n",
      "summary_en": "This project aims at the exploitation of quantum interference effects that occur on a molecular scale to obtain molecular electronic devices with improved characteristics. There is a widespread interest in the study of molecular electronics at present since the dimensions of the active element in integrated circuits are rapidly approaching those of single molecules. Although considerable progress has been made in this field, the design of molecular devices often disregards quantum interference effects that are operative on the scale of singe molecules. In this project these interference effects will be explicitly considered with the aim to use them in a functional way. In this way it will be possible to make molecular transistors with very high on/off ratios and fast switching speeds.\n\nThe interference effects will be studied by considering charge transfer in donor-bridge-acceptor systems where charge transfer occurs upon excitation with a short laser pulse. The molecular bridge will explicitly be chosen to exhibit interference effects on charge transfer. Examples of such bridges are molecules containing two separate pathways for charge transfer (a molecular Mach-Zehnder interferometer) or systems with a dangling reflecting ?stub? (molecular quantum interference transistor). Charge transfer in such systems will be studied experimentally using time-resolved spectroscopic techniques, and theoretically using quantum chemical simulations. The research proposed here will lead to a profound fundamental understanding of quantum interference effects in molecular electronics and quantitative knowledge on the effects of dephasing.\n\nThe approach of studying molecular electronic components through spectroscopic characterization of charge transfer in donor-bridge-acceptor systems represents a strong and unique addition to the considerable effort on molecular scale electronics in the Netherlands. The applicant is excellently positioned to pursue such a program given his proven track record in combining spectroscopic experimental work with computational chemistry to study charge and excited state dynamics.\n\n",
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          "last_name": "Tarkuc",
          "degree_pre_nominal": "dr.",
          "initials": "S.",
          "first_name": "Simge",
          "organisation": "Technische Universiteit Delft",
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          "last_name": "Grozema",
          "degree_pre_nominal": "prof. dr.",
          "initials": "F.C.",
          "first_name": "Ferdinand",
          "organisation": "Technische Universiteit Delft||Faculteit Technische Natuurwetenschappen||Chemical Engineering||Anorganische Chemie",
          "organisation_id": 81244,
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          "initials": "F.C.",
          "first_name": "Ferdinand",
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          "first_name": "Ferdinand",
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